Ultraviolet photodissociation of methanethiol (CH3SH): Revealing an S(1D) atom elimination channel

Chem. Sci., 2025, Accepted Manuscript
DOI: 10.1039/D5SC04716A, Edge Article

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&nbsp This article is licensed under a Creative Commons Attribution 3.0 Unported Licence.

Yucheng Wu, Shunyang Zhou, Zijie Luo, Shuaikang Yang, Zhenxing Li, Yongxin Dong, Wei Hua, Quan Shuai, Dongxu Dai, Michael N R Ashfold, Kaijun Yuan, Xueming Yang
We report time-sliced velocity map imaging studies of the methyl (CH₃) and electronically excited sulfur (S(¹D)) fragments formed following photoexcitation of jet-cooled CH₃SH molecules in the 2¹A”−X¹A’absorption band (i.e. at…
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